TY - JOUR
T1 - An Unexpected Seasonal Cycle in U.S. Oil and Gas Methane Emissions
AU - Hu, Lei
AU - Andrews, Arlyn E.
AU - Montzka, Stephen A.
AU - Miller, Scot M.
AU - Bruhwiler, Lori
AU - Oh, Youmi
AU - Sweeney, Colm
AU - Miller, John B.
AU - McKain, Kathryn
AU - Ibarra Espinosa, Sergio
AU - Davis, Kenneth
AU - Miles, Natasha
AU - Mountain, Marikate
AU - Lan, Xin
AU - Crotwell, Andy
AU - Madronich, Monica
AU - Mefford, Thomas
AU - Michel, Sylvia
AU - Houwelling, Sander
N1 - Publisher Copyright:
© 2025 The Authors. Published by American Chemical Society.
PY - 2025/5/27
Y1 - 2025/5/27
N2 - Accurate quantification of methane (CH4) emissions is essential for understanding changes in its atmospheric abundance. Atmospheric observations can supply independent emission information that complements and strengthens inventory-based estimates. In this study, we quantified annual and monthly U.S. CH4 emissions in 2008-2021 using inverse modeling of ground and airborne measurements at sites across the U.S. with 10-12 km atmospheric transport simulations. While the magnitude, spatial distribution, and trend of the estimated CH4 emissions align with some previous studies, our results reveal an unexpected seasonal cycle in CH4 emissions from the oil and gas sector, where wintertime emissions are about 40 (20-50, 2σ) % higher than summertime. This seasonality is supported by methane and propane measurements at these same sites, as well as methane isotope measurements made from an independent aircraft campaign over the U.S. Although the exact cause of this emission seasonality is unclear, its spatial distribution indicates that the enhanced CH4 emissions are primarily from natural gas production regions, and to a lesser extent, from natural gas consumption in winter.
AB - Accurate quantification of methane (CH4) emissions is essential for understanding changes in its atmospheric abundance. Atmospheric observations can supply independent emission information that complements and strengthens inventory-based estimates. In this study, we quantified annual and monthly U.S. CH4 emissions in 2008-2021 using inverse modeling of ground and airborne measurements at sites across the U.S. with 10-12 km atmospheric transport simulations. While the magnitude, spatial distribution, and trend of the estimated CH4 emissions align with some previous studies, our results reveal an unexpected seasonal cycle in CH4 emissions from the oil and gas sector, where wintertime emissions are about 40 (20-50, 2σ) % higher than summertime. This seasonality is supported by methane and propane measurements at these same sites, as well as methane isotope measurements made from an independent aircraft campaign over the U.S. Although the exact cause of this emission seasonality is unclear, its spatial distribution indicates that the enhanced CH4 emissions are primarily from natural gas production regions, and to a lesser extent, from natural gas consumption in winter.
UR - https://www.scopus.com/pages/publications/105005088644
UR - https://www.scopus.com/pages/publications/105005088644#tab=citedBy
U2 - 10.1021/acs.est.4c14090
DO - 10.1021/acs.est.4c14090
M3 - Article
C2 - 40366056
AN - SCOPUS:105005088644
SN - 0013-936X
VL - 59
SP - 9968
EP - 9979
JO - Environmental Science and Technology
JF - Environmental Science and Technology
IS - 20
ER -