The contributions of induced-multipole and electron overlap effects to the third-order Raman response were studied. A model was constructed on the polarizability of carbon disulfide dimers using polarizabilities from accurate time-dependent density functional theory calculations. The model was used to calculate the third-order time-domain Raman response of liquid carbon disulfide.
All Science Journal Classification (ASJC) codes
- Physics and Astronomy(all)
- Physical and Theoretical Chemistry