Disentangling the intertwined orders in a magnetic kagome metal

Ji Seop Oh, Ananya Biswas, Mason L. Klemm, Hengxin Tan, Yaofeng Xie, Bin Gao, Makoto Hashimoto, Donghui Lu, Binghai Yan, Pengcheng Dai, Robert J. Birgeneau, Ming Yi

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

Intertwined orders appear when multiple orders are strongly interacting, and kagome metals have emerged as new platforms to explore exotic phases. FeGe has been found to develop a charge density wave (CDW) order within magnetic phase, suggesting an intricate interplay of the lattice, charge, and spin degrees of freedom. Recently, postgrowth annealing has been proposed to tune the CDW order from long-range to complete suppression, offering a tuning knob for the CDW order. Here, by comparing the electronic structures of FeGe subjected to different annealing conditions and distinct CDW properties, we report spectral evolution associated with the lattice and spin degrees of freedom. We find band evolution linked to a spin density wave (SDW) order present in both samples with and without CDW order, and another evolution connected to the lattice distortions that onset with the long-range CDW order and revert with the SDW order. Our results reveal a rare competitive cooperation of the lattice, spin, and charge in FeGe.

Original languageEnglish (US)
Article numbereadt2195
JournalScience Advances
Volume11
Issue number27
DOIs
StatePublished - Jul 4 2025

All Science Journal Classification (ASJC) codes

  • General

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