TY - JOUR
T1 - Electrochemical properties of Gd(III) ions in LiCl-KCl-GdCl3 at 723–1023 K
AU - Baldivieso, Stephanie Castro
AU - Smith, Nathan D.
AU - Liu, Zi Kui
AU - Kim, Hojong
N1 - Publisher Copyright:
© 2023 Elsevier B.V.
PY - 2023/7/1
Y1 - 2023/7/1
N2 - Electrochemical behavior of Gd(III) ions in molten LiCl-KCl-GdCl3 was investigated at 723–1023 K via cyclic voltammetry using tungsten as a working electrode, Gd-Bi (mole fraction, xGd = 0.16) as a reference electrode, and Gd-Bi (xGd = 0.02) as a counter electrode. A single reduction–oxidation wave was observed, confirming a single-step, 3-electron transfer Gd(III)/Gd transition. The cathodic peak potential exhibited minimal change (<13 mV) over a wide range of scan rates (0.05–0.30 V s−1), indicating facile charge transfer kinetics (i.e., a reversible electrode process). A nucleation overpotential associated with solid Gd deposition was observable at low temperatures (T < 823 K). The mass transport properties of Gd(III) ions were estimated using the Berzins and Delahay relation based on diffusion-limiting peak current. The diffusivity values were determined to be DGd(III) = 0.5–2.7 × 10−5 cm2 s−1 at 723–1023 K with an associated activation energy of Ea = 33.9 (±1.0) kJ mol−1. The two-phase [liquid + GdBi] Gd-Bi alloy reference electrode experienced less than 0.5 mV of drift over 5 days of repeated electrochemical measurements, indicating high stability.
AB - Electrochemical behavior of Gd(III) ions in molten LiCl-KCl-GdCl3 was investigated at 723–1023 K via cyclic voltammetry using tungsten as a working electrode, Gd-Bi (mole fraction, xGd = 0.16) as a reference electrode, and Gd-Bi (xGd = 0.02) as a counter electrode. A single reduction–oxidation wave was observed, confirming a single-step, 3-electron transfer Gd(III)/Gd transition. The cathodic peak potential exhibited minimal change (<13 mV) over a wide range of scan rates (0.05–0.30 V s−1), indicating facile charge transfer kinetics (i.e., a reversible electrode process). A nucleation overpotential associated with solid Gd deposition was observable at low temperatures (T < 823 K). The mass transport properties of Gd(III) ions were estimated using the Berzins and Delahay relation based on diffusion-limiting peak current. The diffusivity values were determined to be DGd(III) = 0.5–2.7 × 10−5 cm2 s−1 at 723–1023 K with an associated activation energy of Ea = 33.9 (±1.0) kJ mol−1. The two-phase [liquid + GdBi] Gd-Bi alloy reference electrode experienced less than 0.5 mV of drift over 5 days of repeated electrochemical measurements, indicating high stability.
UR - http://www.scopus.com/inward/record.url?scp=85153674262&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=85153674262&partnerID=8YFLogxK
U2 - 10.1016/j.jelechem.2023.117482
DO - 10.1016/j.jelechem.2023.117482
M3 - Article
AN - SCOPUS:85153674262
SN - 1572-6657
VL - 940
JO - Journal of Electroanalytical Chemistry
JF - Journal of Electroanalytical Chemistry
M1 - 117482
ER -