TY - JOUR
T1 - Eliminating Surface Oxides of Superconducting Circuits with Noble Metal Encapsulation
AU - Chang, Ray D.
AU - Shumiya, Nana
AU - McLellan, Russell A.
AU - Zhang, Yifan
AU - Bland, Matthew P.
AU - Bahrami, Faranak
AU - Mun, Junsik
AU - Zhou, Chenyu
AU - Kisslinger, Kim
AU - Cheng, Guangming
AU - Smitham, Basil M.
AU - Pakpour-Tabrizi, Alexander C.
AU - Yao, Nan
AU - Zhu, Yimei
AU - Liu, Mingzhao
AU - Cava, Robert J.
AU - Gopalakrishnan, Sarang
AU - Houck, Andrew A.
AU - De Leon, Nathalie P.
N1 - Publisher Copyright:
© 2025 American Physical Society.
PY - 2025/3/7
Y1 - 2025/3/7
N2 - The lifetime of superconducting qubits is limited by dielectric loss, and a major source of dielectric loss is the native oxide present at the surface of the superconducting metal. Specifically, tantalum-based superconducting qubits have been demonstrated with record lifetimes, but a major source of loss is the presence of two-level systems in the surface tantalum oxide. Here, we demonstrate a strategy for avoiding oxide formation by encapsulating the tantalum with noble metals that do not form native oxide. By depositing a few nanometers of Au or AuPd alloy before breaking vacuum, we completely suppress tantalum oxide formation. Microwave loss measurements of superconducting resonators reveal that the noble metal is proximitized, with a superconducting gap over 80% of the bare tantalum at thicknesses where the oxide is fully suppressed. Our findings suggest that losses in resonators fabricated by subtractive etching are dominated by oxides on the sidewalls, pointing to total surface encapsulation by additive fabrication as a promising strategy for eliminating surface oxide two-level system loss in superconducting qubits.
AB - The lifetime of superconducting qubits is limited by dielectric loss, and a major source of dielectric loss is the native oxide present at the surface of the superconducting metal. Specifically, tantalum-based superconducting qubits have been demonstrated with record lifetimes, but a major source of loss is the presence of two-level systems in the surface tantalum oxide. Here, we demonstrate a strategy for avoiding oxide formation by encapsulating the tantalum with noble metals that do not form native oxide. By depositing a few nanometers of Au or AuPd alloy before breaking vacuum, we completely suppress tantalum oxide formation. Microwave loss measurements of superconducting resonators reveal that the noble metal is proximitized, with a superconducting gap over 80% of the bare tantalum at thicknesses where the oxide is fully suppressed. Our findings suggest that losses in resonators fabricated by subtractive etching are dominated by oxides on the sidewalls, pointing to total surface encapsulation by additive fabrication as a promising strategy for eliminating surface oxide two-level system loss in superconducting qubits.
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U2 - 10.1103/PhysRevLett.134.097001
DO - 10.1103/PhysRevLett.134.097001
M3 - Article
C2 - 40131031
AN - SCOPUS:86000355062
SN - 0031-9007
VL - 134
JO - Physical review letters
JF - Physical review letters
IS - 9
M1 - 097001
ER -