Fast and Efficient Preparation of Exfoliated 2H MoS2 Nanosheets by Sonication-Assisted Lithium Intercalation and Infrared Laser-Induced 1T to 2H Phase Reversion

Xiaobin Fan, Pengtao Xu, Dekai Zhou, Yifan Sun, Yuguang C. Li, Minh An T. Nguyen, Mauricio Terrones, Thomas E. Mallouk

Research output: Contribution to journalArticlepeer-review

630 Scopus citations

Abstract

Exfoliated 2H molybdenum disulfide (MoS2) has unique properties and potential applications in a wide range of fields, but corresponding studies have been hampered by the lack of effective routes to it in bulk quantities. This study presents a rapid and efficient route to obtain exfoliated 2H MoS2, which combines fast sonication-assisted lithium intercalation and infrared (IR) laser-induced phase reversion. We found that the complete lithium intercalation of MoS2 with butyllithium could be effected within 1.5 h with the aid of sonication. The 2H to 1T phase transition that occurs during the lithium intercalation could be also reversed by IR laser irradiation with a DVD optical drive.

Original languageEnglish (US)
Pages (from-to)5956-5960
Number of pages5
JournalNano letters
Volume15
Issue number9
DOIs
StatePublished - Sep 9 2015

All Science Journal Classification (ASJC) codes

  • Bioengineering
  • General Chemistry
  • General Materials Science
  • Condensed Matter Physics
  • Mechanical Engineering

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