TY - JOUR
T1 - Good plasmons in a bad metal
AU - Ruta, Francesco L.
AU - Shao, Yinming
AU - Acharya, Swagata
AU - Mu, Anqi
AU - Jo, Na Hyun
AU - Ryu, Sae Hee
AU - Balatsky, Daria
AU - Su, Yifan
AU - Pashov, Dimitar
AU - Kim, Brian S.Y.
AU - Katsnelson, Mikhail I.
AU - Analytis, James G.
AU - Rotenberg, Eli
AU - Millis, Andrew J.
AU - van Schilfgaarde, Mark
AU - Basov, D. N.
PY - 2025/1/2
Y1 - 2025/1/2
N2 - Correlated metals may exhibit unusually high resistivity that increases linearly in temperature, breaking through the Mott-Ioffe-Regel bound, above which coherent quasiparticles are destroyed. The fate of collective charge excitations, or plasmons, in these systems is a subject of debate. Several studies have suggested that plasmons are overdamped, whereas other studies have detected propagating plasmons. In this work, we present direct nano-optical images of low-loss hyperbolic plasmon polaritons (HPPs) in the correlated van der Waals metal MoOCl2. HPPs are plasmon-photon modes that waveguide through extremely anisotropic media and are remarkably long-lived in MoOCl2. Photoemission data presented here reveal a highly anisotropic Fermi surface, reconstructed and made partly incoherent, likely through electronic interactions as explained by many-body theory. HPPs remain long-lived despite this, revealing previously unseen imprints of many-body effects on plasmonic collective modes.
AB - Correlated metals may exhibit unusually high resistivity that increases linearly in temperature, breaking through the Mott-Ioffe-Regel bound, above which coherent quasiparticles are destroyed. The fate of collective charge excitations, or plasmons, in these systems is a subject of debate. Several studies have suggested that plasmons are overdamped, whereas other studies have detected propagating plasmons. In this work, we present direct nano-optical images of low-loss hyperbolic plasmon polaritons (HPPs) in the correlated van der Waals metal MoOCl2. HPPs are plasmon-photon modes that waveguide through extremely anisotropic media and are remarkably long-lived in MoOCl2. Photoemission data presented here reveal a highly anisotropic Fermi surface, reconstructed and made partly incoherent, likely through electronic interactions as explained by many-body theory. HPPs remain long-lived despite this, revealing previously unseen imprints of many-body effects on plasmonic collective modes.
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U2 - 10.1126/science.adr5926
DO - 10.1126/science.adr5926
M3 - Article
C2 - 39946465
AN - SCOPUS:85218827486
SN - 0036-8075
VL - 387
SP - 786
EP - 791
JO - Science (New York, N.Y.)
JF - Science (New York, N.Y.)
IS - 6735
ER -