Good plasmons in a bad metal

  • Francesco L. Ruta
  • , Yinming Shao
  • , Swagata Acharya
  • , Anqi Mu
  • , Na Hyun Jo
  • , Sae Hee Ryu
  • , Daria Balatsky
  • , Yifan Su
  • , Dimitar Pashov
  • , Brian S.Y. Kim
  • , Mikhail I. Katsnelson
  • , James G. Analytis
  • , Eli Rotenberg
  • , Andrew J. Millis
  • , Mark van Schilfgaarde
  • , D. N. Basov

Research output: Contribution to journalArticlepeer-review

9 Scopus citations

Abstract

Correlated metals may exhibit unusually high resistivity that increases linearly in temperature, breaking through the Mott-Ioffe-Regel bound, above which coherent quasiparticles are destroyed. The fate of collective charge excitations, or plasmons, in these systems is a subject of debate. Several studies have suggested that plasmons are overdamped, whereas other studies have detected propagating plasmons. In this work, we present direct nano-optical images of low-loss hyperbolic plasmon polaritons (HPPs) in the correlated van der Waals metal MoOCl2. HPPs are plasmon-photon modes that waveguide through extremely anisotropic media and are remarkably long-lived in MoOCl2. Photoemission data presented here reveal a highly anisotropic Fermi surface, reconstructed and made partly incoherent, likely through electronic interactions as explained by many-body theory. HPPs remain long-lived despite this, revealing previously unseen imprints of many-body effects on plasmonic collective modes.

Original languageEnglish (US)
Pages (from-to)786-791
Number of pages6
JournalScience
Volume387
Issue number6735
DOIs
StatePublished - Feb 14 2025

All Science Journal Classification (ASJC) codes

  • General

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