Abstract
Here, we present a temperature (T) dependent comparison between field-effect and Hall mobilities in field-effect transistors based on few-layered WSe2 exfoliated onto SiO2. Without dielectric engineering and beyond a T-dependent threshold gate-voltage, we observe maximum hole mobilities approaching 350 cm2 /Vs at T = 300 K. The hole Hall mobility reaches a maximum value of 650 cm2 /Vs as T is lowered below ∼150 K, indicating that insofar WSe2 -based field-effect transistors (FETs) display the largest Hall mobilities among the transition metal dichalcogenides. The gate capacitance, as extracted from the Hall-effect, reveals the presence of spurious charges in the channel, while the two-terminal sheet resistivity displays two-dimensional variable-range hopping behavior, indicating carrier localization induced by disorder at the interface between WSe2 and SiO2. We argue that improvements in the fabrication protocols as, for example, the use of a substrate free of dangling bonds are likely to produce WSe2-based FETs displaying higher room temperature mobilities, i.e. approaching those of p-doped Si, which would make it a suitable candidate for high performance opto-electronics.
| Original language | English (US) |
|---|---|
| Article number | 8979 |
| Journal | Scientific reports |
| Volume | 5 |
| DOIs | |
| State | Published - Mar 11 2015 |
All Science Journal Classification (ASJC) codes
- General