Investigation of dielectric and piezoelectric properties in Pb(Ni1/3Nb2/3)O3-PbHfO3-PbTi O3 ternary system

H. Tang; M. F. Zhang; S. J. Zhang; Y. J. Feng; F. Li; T. R. Shrout

doi:10.1016/j.jeurceramsoc.2013.04.010

Investigation of dielectric and piezoelectric properties in Pb(Ni_1/3Nb_2/3)O₃-PbHfO₃-PbTi O₃ ternary system

H. Tang, M. F. Zhang, S. J. Zhang, Y. J. Feng, F. Li, T. R. Shrout

Materials Research Institute (MRI)

Research output: Contribution to journal › Article › peer-review

68 Scopus citations

Abstract

The dielectric and piezoelectric properties were investigated in the (1-x)Pb(Hf_1-yTi_y)O₃-xPb(Ni_1/3Nb_2/3)O₃ (PNN-PHT, x=0.05-0.50, y=0.55-0.70) ternary system. The morphotropic phase boundary (MPB) was determined by X-ray powder diffraction analysis. Isothermal map of Curie temperature (T_C) related to the compositions in the phase diagram was obtained. The optimum dielectric and piezoelectric properties were achieved in ceramics with the MPB compositions, with the maxima values being on the order of 6000 and 970pC/N, respectively. Rayleigh analysis was used to study the extrinsic contribution (domain wall motion) in PNN-PHT system, where the extrinsic contribution was found to be ~30% for composition 0.49PNN-0.51PHT(30/70), showing a high nonlinearity.

Original language	English (US)
Pages (from-to)	2491-2497
Number of pages	7
Journal	Journal of the European Ceramic Society
Volume	33
Issue number	13-14
DOIs	https://doi.org/10.1016/j.jeurceramsoc.2013.04.010
State	Published - Nov 2013

All Science Journal Classification (ASJC) codes

Ceramics and Composites
Materials Chemistry

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10.1016/j.jeurceramsoc.2013.04.010

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@article{76d38f5320dd4be09c31b1e0445edb40,

title = "Investigation of dielectric and piezoelectric properties in Pb(Ni1/3Nb2/3)O3-PbHfO3-PbTi O3 ternary system",

abstract = "The dielectric and piezoelectric properties were investigated in the (1-x)Pb(Hf1-yTiy)O3-xPb(Ni1/3Nb2/3)O3 (PNN-PHT, x=0.05-0.50, y=0.55-0.70) ternary system. The morphotropic phase boundary (MPB) was determined by X-ray powder diffraction analysis. Isothermal map of Curie temperature (TC) related to the compositions in the phase diagram was obtained. The optimum dielectric and piezoelectric properties were achieved in ceramics with the MPB compositions, with the maxima values being on the order of 6000 and 970pC/N, respectively. Rayleigh analysis was used to study the extrinsic contribution (domain wall motion) in PNN-PHT system, where the extrinsic contribution was found to be ~30% for composition 0.49PNN-0.51PHT(30/70), showing a high nonlinearity.",

author = "H. Tang and Zhang, {M. F.} and Zhang, {S. J.} and Feng, {Y. J.} and F. Li and Shrout, {T. R.}",

note = "Funding Information: The authors Hua Tang and Mingfu Zhang want to acknowledge the supports from the China Scholarship Council . ",

year = "2013",

month = nov,

doi = "10.1016/j.jeurceramsoc.2013.04.010",

language = "English (US)",

volume = "33",

pages = "2491--2497",

journal = "Journal of the European Ceramic Society",

issn = "0955-2219",

publisher = "Elsevier B.V.",

number = "13-14",

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TY - JOUR

T1 - Investigation of dielectric and piezoelectric properties in Pb(Ni1/3Nb2/3)O3-PbHfO3-PbTi O3 ternary system

AU - Tang, H.

AU - Zhang, M. F.

AU - Zhang, S. J.

AU - Feng, Y. J.

AU - Li, F.

AU - Shrout, T. R.

N1 - Funding Information: The authors Hua Tang and Mingfu Zhang want to acknowledge the supports from the China Scholarship Council .

PY - 2013/11

Y1 - 2013/11

N2 - The dielectric and piezoelectric properties were investigated in the (1-x)Pb(Hf1-yTiy)O3-xPb(Ni1/3Nb2/3)O3 (PNN-PHT, x=0.05-0.50, y=0.55-0.70) ternary system. The morphotropic phase boundary (MPB) was determined by X-ray powder diffraction analysis. Isothermal map of Curie temperature (TC) related to the compositions in the phase diagram was obtained. The optimum dielectric and piezoelectric properties were achieved in ceramics with the MPB compositions, with the maxima values being on the order of 6000 and 970pC/N, respectively. Rayleigh analysis was used to study the extrinsic contribution (domain wall motion) in PNN-PHT system, where the extrinsic contribution was found to be ~30% for composition 0.49PNN-0.51PHT(30/70), showing a high nonlinearity.

AB - The dielectric and piezoelectric properties were investigated in the (1-x)Pb(Hf1-yTiy)O3-xPb(Ni1/3Nb2/3)O3 (PNN-PHT, x=0.05-0.50, y=0.55-0.70) ternary system. The morphotropic phase boundary (MPB) was determined by X-ray powder diffraction analysis. Isothermal map of Curie temperature (TC) related to the compositions in the phase diagram was obtained. The optimum dielectric and piezoelectric properties were achieved in ceramics with the MPB compositions, with the maxima values being on the order of 6000 and 970pC/N, respectively. Rayleigh analysis was used to study the extrinsic contribution (domain wall motion) in PNN-PHT system, where the extrinsic contribution was found to be ~30% for composition 0.49PNN-0.51PHT(30/70), showing a high nonlinearity.

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U2 - 10.1016/j.jeurceramsoc.2013.04.010

DO - 10.1016/j.jeurceramsoc.2013.04.010

M3 - Article

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SN - 0955-2219

VL - 33

SP - 2491

EP - 2497

JO - Journal of the European Ceramic Society

JF - Journal of the European Ceramic Society

IS - 13-14

ER -

Investigation of dielectric and piezoelectric properties in Pb(Ni_1/3Nb_2/3)O₃-PbHfO₃-PbTi O₃ ternary system

Abstract

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