TY - JOUR
T1 - Nano-aluminum flame spread with fingering combustion instabilities
AU - Malchi, J. Y.
AU - Yetter, R. A.
AU - Son, S. F.
AU - Risha, G. A.
N1 - Funding Information:
This work was sponsored by the US Army Research Office under the Multi-University Research Initiative under Contract No. W911NF-04-1-0178. The support and encouragement provided by Dr. David Mann and Dr. Kevin L. McNesby are gratefully acknowledged. S.F.S. is supported by Los Alamos National Laboratory (LANL), which is operated by the University of California for the US Department of Energy under the contract W-7405-ENG-36. The authors thank personnel at LANL, specifically Mr. Ed Roemer for the SEM micrographs of the particles and Mr. Eric Sanders for supplying the 38 nm aluminum particles.
Copyright:
Copyright 2021 Elsevier B.V., All rights reserved.
PY - 2007
Y1 - 2007
N2 - Three consecutive modes of flame propagation were observed over a bed of nano-aluminum burning with a counter-flowing oxidizer of 20% oxygen and 80% argon by volume, each displaying significantly different characteristics. The first mode of propagation was the focus of this study and was examined within the critical Rayleigh and Peclet number regime where three-dimensional buoyancy effects were hindered and the fingering thermal-diffusive instability occurred. Fingering flame spread was observed and characterized for various Peclet numbers, top plate heights and particle sizes to gain a better understanding of the reaction mechanism associated with the combustion of nano-particles in close contact. Results indicate that the first mode of flame propagation over a bed of nano-aluminum has spread rates an order of magnitude greater than that of cellulose fuels. However, similar trends occur when varying the Peclet number and the height of the top plate. Furthermore, faster propagation speeds occur with smaller particles because of their increased specific surface area. The widths of the fingers grow and more of the surface is burned with increasing particle size due to the longer time scale available for lateral growth.
AB - Three consecutive modes of flame propagation were observed over a bed of nano-aluminum burning with a counter-flowing oxidizer of 20% oxygen and 80% argon by volume, each displaying significantly different characteristics. The first mode of propagation was the focus of this study and was examined within the critical Rayleigh and Peclet number regime where three-dimensional buoyancy effects were hindered and the fingering thermal-diffusive instability occurred. Fingering flame spread was observed and characterized for various Peclet numbers, top plate heights and particle sizes to gain a better understanding of the reaction mechanism associated with the combustion of nano-particles in close contact. Results indicate that the first mode of flame propagation over a bed of nano-aluminum has spread rates an order of magnitude greater than that of cellulose fuels. However, similar trends occur when varying the Peclet number and the height of the top plate. Furthermore, faster propagation speeds occur with smaller particles because of their increased specific surface area. The widths of the fingers grow and more of the surface is burned with increasing particle size due to the longer time scale available for lateral growth.
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U2 - 10.1016/j.proci.2006.08.046
DO - 10.1016/j.proci.2006.08.046
M3 - Conference article
AN - SCOPUS:34548791160
SN - 1540-7489
VL - 31 II
SP - 2617
EP - 2624
JO - Proceedings of the Combustion Institute
JF - Proceedings of the Combustion Institute
IS - 2
T2 - 31st International Symposium on Combustion
Y2 - 5 August 2006 through 11 August 2006
ER -