Near-field imaging of plasmonic nanopatch antennas with integrated semiconductor quantum dots

Vasudevan Iyer, Yoong Sheng Phang, Andrew Butler, Jiyang Chen, Brian Lerner, Christos Argyropoulos, Thang Hoang, Benjamin Lawrie

Research output: Contribution to journalArticlepeer-review

11 Scopus citations

Abstract

Plasmonic nanopatch antennas that incorporate dielectric gaps hundreds of picometers to several nanometers thick have drawn increasing attention over the past decade because they confine electromagnetic fields to grossly sub-diffraction-limited volumes. Substantial control over the optical properties of excitons and color centers confined within these plasmonic cavities has already been demonstrated with far-field optical spectroscopies, but near-field optical spectroscopies are essential for an improved understanding of the plasmon-emitter interaction at the nanoscale. Here, we characterize the intensity and phase-resolved plasmonic response of isolated nanopatch antennas by cathodoluminescence microscopy. Furthermore, we explore the distinction between optical and electron beam spectroscopies of coupled plasmon-exciton heterostructures to identify constraints and opportunities for future nanoscale characterization and control of hybrid nanophotonic structures. While we observe substantial Purcell enhancement in time-resolved photoluminescence spectroscopies, negligible Purcell enhancement is observed in cathodoluminescence spectroscopies of hybrid nanophotonic structures. The substantial differences in measured Purcell enhancement for electron beam and laser excitation can be understood as a result of the different selection rules for these complementary experiments. These results provide a fundamentally new understanding of near-field plasmon-exciton interactions in nanopatch antennas, which is essential for myriad emerging quantum photonic devices.

Original languageEnglish (US)
Article number106103
JournalAPL Photonics
Volume6
Issue number10
DOIs
StatePublished - Oct 1 2021

All Science Journal Classification (ASJC) codes

  • Atomic and Molecular Physics, and Optics
  • Computer Networks and Communications

Fingerprint

Dive into the research topics of 'Near-field imaging of plasmonic nanopatch antennas with integrated semiconductor quantum dots'. Together they form a unique fingerprint.

Cite this