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Nonvanishing Subgap Photocurrent as a Probe of Lifetime Effects

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Abstract

For semiconductors and insulators, it is commonly believed that in-gap transitions into nonlocalized states are smoothly suppressed in the clean limit; i.e., at zero temperature, their contribution vanishes due to the unavailability of states. We present a novel type of subgap response which shows that this intuition does not generalize beyond linear response. Namely, we find that the dc current due to the bulk photovoltaic effect can be finite and mostly temperature independent in an allowed window of subgap transitions. We expect that a moderate range of excitation energies lies between the bulk energy gap and the mobility edge where this effect is observable. Using a simplified relaxation time model for the band broadening, we find the subgap dc current to be temperature independent for noninteracting systems but temperature dependent for strongly interacting systems. Thus, the subgap response may be used to distinguish whether a state is single-particle localized or many-body localized.

Original languageEnglish (US)
Article number227205
JournalPhysical review letters
Volume125
Issue number22
DOIs
StatePublished - Nov 25 2020

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 7 - Affordable and Clean Energy
    SDG 7 Affordable and Clean Energy

All Science Journal Classification (ASJC) codes

  • General Physics and Astronomy

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