Optical properties and dispersions of rhombohedral 0.24Pb(In 1/2Nb1/2)O3-0.49Pb(Mg1/3Nb 2/3)O3-0.27PbTiO3 single domain single crystal

Fengmin Wu; Bin Yang; Enwei Sun; Wenlong Yang; Wenwu Cao

doi:10.1016/j.optmat.2013.09.020

Optical properties and dispersions of rhombohedral 0.24Pb(In _1/2Nb_1/2)O₃-0.49Pb(Mg_1/3Nb _2/3)O₃-0.27PbTiO₃ single domain single crystal

Fengmin Wu, Bin Yang, Enwei Sun, Wenlong Yang, Wenwu Cao

Research output: Contribution to journal › Article › peer-review

12 Scopus citations

Abstract

The ternary relaxor-based ferroelectric single crystal 0.24Pb(In _1/2Nb_1/2)O₃-0.49Pb(Mg_1/3Nb _2/3)O₃-0.27PbTiO₃ (0.24PIN-0.49PMN-0.27PT) poled along [1 1 1]_c has remarkable optical properties. Its Curie temperature T_c is 168 C determined by the dielectric constant measurement. Optical transmission spectra were recorded at both room temperature and 200 C. The optical absorption edge at 200 C has an obvious red-shift compared with that at room temperature, the bandgaps were determined to be E_g = 3.18 eV and 2.95 eV at room temperature and at 200 C, respectively. Parameters for the Varshini equations are: E_g(0) = 3.27 eV, a = 1.62 × 10^-3 meV/K and b = 1315 K. We have obtained the refractive indices and the extinction coefficients in the single-domain state. The parameters of room temperature monomial Sellmeier oscillator were also derived.

Original language	English (US)
Pages (from-to)	342-345
Number of pages	4
Journal	Optical Materials
Volume	36
Issue number	2
DOIs	https://doi.org/10.1016/j.optmat.2013.09.020
State	Published - Dec 2013

All Science Journal Classification (ASJC) codes

Electronic, Optical and Magnetic Materials
General Computer Science
Atomic and Molecular Physics, and Optics
Spectroscopy
Physical and Theoretical Chemistry
Organic Chemistry
Inorganic Chemistry
Electrical and Electronic Engineering

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10.1016/j.optmat.2013.09.020

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@article{ab675002b42e49079bf1761bb7087f94,

title = "Optical properties and dispersions of rhombohedral 0.24Pb(In 1/2Nb1/2)O3-0.49Pb(Mg1/3Nb 2/3)O3-0.27PbTiO3 single domain single crystal",

abstract = "The ternary relaxor-based ferroelectric single crystal 0.24Pb(In 1/2Nb1/2)O3-0.49Pb(Mg1/3Nb 2/3)O3-0.27PbTiO3 (0.24PIN-0.49PMN-0.27PT) poled along [1 1 1]c has remarkable optical properties. Its Curie temperature Tc is 168 C determined by the dielectric constant measurement. Optical transmission spectra were recorded at both room temperature and 200 C. The optical absorption edge at 200 C has an obvious red-shift compared with that at room temperature, the bandgaps were determined to be Eg = 3.18 eV and 2.95 eV at room temperature and at 200 C, respectively. Parameters for the Varshini equations are: Eg(0) = 3.27 eV, a = 1.62 × 10-3 meV/K and b = 1315 K. We have obtained the refractive indices and the extinction coefficients in the single-domain state. The parameters of room temperature monomial Sellmeier oscillator were also derived.",

author = "Fengmin Wu and Bin Yang and Enwei Sun and Wenlong Yang and Wenwu Cao",

note = "Funding Information: This research was supported by the National key Basic Research Program of China (973 Program) under Grant No. 2013CB632900 , the NIH under Grant No. P41-EB2182 , the National Nature Science Foundation of China under Grant No. 10704021 , the Young Foundation of Harbin University of Science and Technology under Grant No. 2011YF007 , High quality PIN-PMN-PT single crystals were provided by H. C. Materials Inc, Bolingbrook, IL, USA. ",

year = "2013",

month = dec,

doi = "10.1016/j.optmat.2013.09.020",

language = "English (US)",

volume = "36",

pages = "342--345",

journal = "Optical Materials",

issn = "0925-3467",

publisher = "Elsevier B.V.",

number = "2",

}

TY - JOUR

T1 - Optical properties and dispersions of rhombohedral 0.24Pb(In 1/2Nb1/2)O3-0.49Pb(Mg1/3Nb 2/3)O3-0.27PbTiO3 single domain single crystal

AU - Wu, Fengmin

AU - Yang, Bin

AU - Sun, Enwei

AU - Yang, Wenlong

AU - Cao, Wenwu

N1 - Funding Information: This research was supported by the National key Basic Research Program of China (973 Program) under Grant No. 2013CB632900 , the NIH under Grant No. P41-EB2182 , the National Nature Science Foundation of China under Grant No. 10704021 , the Young Foundation of Harbin University of Science and Technology under Grant No. 2011YF007 , High quality PIN-PMN-PT single crystals were provided by H. C. Materials Inc, Bolingbrook, IL, USA.

PY - 2013/12

Y1 - 2013/12

N2 - The ternary relaxor-based ferroelectric single crystal 0.24Pb(In 1/2Nb1/2)O3-0.49Pb(Mg1/3Nb 2/3)O3-0.27PbTiO3 (0.24PIN-0.49PMN-0.27PT) poled along [1 1 1]c has remarkable optical properties. Its Curie temperature Tc is 168 C determined by the dielectric constant measurement. Optical transmission spectra were recorded at both room temperature and 200 C. The optical absorption edge at 200 C has an obvious red-shift compared with that at room temperature, the bandgaps were determined to be Eg = 3.18 eV and 2.95 eV at room temperature and at 200 C, respectively. Parameters for the Varshini equations are: Eg(0) = 3.27 eV, a = 1.62 × 10-3 meV/K and b = 1315 K. We have obtained the refractive indices and the extinction coefficients in the single-domain state. The parameters of room temperature monomial Sellmeier oscillator were also derived.

AB - The ternary relaxor-based ferroelectric single crystal 0.24Pb(In 1/2Nb1/2)O3-0.49Pb(Mg1/3Nb 2/3)O3-0.27PbTiO3 (0.24PIN-0.49PMN-0.27PT) poled along [1 1 1]c has remarkable optical properties. Its Curie temperature Tc is 168 C determined by the dielectric constant measurement. Optical transmission spectra were recorded at both room temperature and 200 C. The optical absorption edge at 200 C has an obvious red-shift compared with that at room temperature, the bandgaps were determined to be Eg = 3.18 eV and 2.95 eV at room temperature and at 200 C, respectively. Parameters for the Varshini equations are: Eg(0) = 3.27 eV, a = 1.62 × 10-3 meV/K and b = 1315 K. We have obtained the refractive indices and the extinction coefficients in the single-domain state. The parameters of room temperature monomial Sellmeier oscillator were also derived.

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SN - 0925-3467

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JO - Optical Materials

JF - Optical Materials

IS - 2

ER -

Optical properties and dispersions of rhombohedral 0.24Pb(In _1/2Nb_1/2)O₃-0.49Pb(Mg_1/3Nb _2/3)O₃-0.27PbTiO₃ single domain single crystal

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