TY - JOUR
T1 - Plasmon Enhanced Quantum Properties of Single Photon Emitters with Hybrid Hexagonal Boron Nitride Silver Nanocube Systems
AU - Dowran, Mohammadjavad
AU - Butler, Andrew
AU - Lamichhane, Suvechhya
AU - Erickson, Adam
AU - Kilic, Ufuk
AU - Liou, Sy Hwang
AU - Argyropoulos, Christos
AU - Laraoui, Abdelghani
N1 - Publisher Copyright:
© 2023 The Authors. Advanced Optical Materials published by Wiley-VCH GmbH.
PY - 2023/8/21
Y1 - 2023/8/21
N2 - Hexagonal boron nitride (hBN) has emerged as a promising ultrathin host of single photon emitters (SPEs) with favorable quantum properties at room temperature, making it a highly desirable element for integrated quantum photonic networks. One major challenge of using these SPEs in such applications is their low quantum efficiency. Recent studies have reported an improvement in quantum efficiency by up to two orders of magnitude when integrating an ensemble of emitters such as boron vacancy defects in multilayered hBN flakes embedded within metallic nanocavities. However, these experiments have not been extended to SPEs and are mainly focused on multiphoton effects. Here, the quantum single-photon properties of hybrid nanophotonic structures composed of SPEs created in ultrathin hBN flakes coupled with plasmonic silver nanocubes (SNCs) are studied. The authors demonstrate 200% plasmonic enhancement of the SPE properties, manifested by a strong increase in the SPE fluorescence. Such enhancement is explained by rigorous numerical simulations where the hBN flake is in direct contact with the SNCs that cause the plasmonic effects. The presented strong and fast single photon emission obtained at room temperature with a compact hybrid nanophotonic platform can be very useful to various emerging applications in quantum optical communications and computing.
AB - Hexagonal boron nitride (hBN) has emerged as a promising ultrathin host of single photon emitters (SPEs) with favorable quantum properties at room temperature, making it a highly desirable element for integrated quantum photonic networks. One major challenge of using these SPEs in such applications is their low quantum efficiency. Recent studies have reported an improvement in quantum efficiency by up to two orders of magnitude when integrating an ensemble of emitters such as boron vacancy defects in multilayered hBN flakes embedded within metallic nanocavities. However, these experiments have not been extended to SPEs and are mainly focused on multiphoton effects. Here, the quantum single-photon properties of hybrid nanophotonic structures composed of SPEs created in ultrathin hBN flakes coupled with plasmonic silver nanocubes (SNCs) are studied. The authors demonstrate 200% plasmonic enhancement of the SPE properties, manifested by a strong increase in the SPE fluorescence. Such enhancement is explained by rigorous numerical simulations where the hBN flake is in direct contact with the SNCs that cause the plasmonic effects. The presented strong and fast single photon emission obtained at room temperature with a compact hybrid nanophotonic platform can be very useful to various emerging applications in quantum optical communications and computing.
UR - https://www.scopus.com/pages/publications/85158123092
UR - https://www.scopus.com/inward/citedby.url?scp=85158123092&partnerID=8YFLogxK
U2 - 10.1002/adom.202300392
DO - 10.1002/adom.202300392
M3 - Article
AN - SCOPUS:85158123092
SN - 2195-1071
VL - 11
JO - Advanced Optical Materials
JF - Advanced Optical Materials
IS - 16
M1 - 2300392
ER -