TY - JOUR
T1 - Scaling Urban Methane Emissions
T2 - Utility of Single-Site Measurements in Five Urban Domains
AU - Mueller, Kimberly L.
AU - Karion, Anna
AU - Lopez-Coto, Israel
AU - Marrs, Julia
AU - Yadav, Vineet
AU - Plant, Genevieve
AU - Pitt, Joseph
AU - Barkley, Zachary R.
AU - Whetstone, James
N1 - Publisher Copyright:
© 2025 The Authors. Published by American Chemical Society
PY - 2025/7/22
Y1 - 2025/7/22
N2 - Urban methane (CH4) missions remain poorly understood due to limited observational constraints. Most estimates rely on bottom-up inventories based on assumed emission factors and activity data or downscaling methods, which often underestimate emissions, sometimes by a factor of 2 or more in United States and European cities. While satellite and mobile observations can improve understanding, they face limitations in spatial resolution, coverage, and frequency. In contrast, fixed in situ measurements calibrated to World Meteorological Organization standards offer high precision continuous data, although with limited spatial coverage due to logistical constraints. This study uses in situ observations from single tower sites in five northeastern United States cities to estimate total urban CH4emissions using a Bayesian scaling factor framework. Despite limited spatial sampling, the approach yields robust emission estimates consistent with other studies. To explore drivers of variability, the analysis examines correlations between inferred emissions and urban characteristics including population, residential gas usage, and infrastructure. Results show that residential building volume outperforms population as a predictor in some regions, highlighting the importance of infrastructure-specific factors. By demonstrating a scalable observation-based approach using minimal sites, this work addresses key gaps in urban CH4monitoring and emphasizes the value of robust measurements and tailored proxies for improving emission estimates in diverse urban settings.
AB - Urban methane (CH4) missions remain poorly understood due to limited observational constraints. Most estimates rely on bottom-up inventories based on assumed emission factors and activity data or downscaling methods, which often underestimate emissions, sometimes by a factor of 2 or more in United States and European cities. While satellite and mobile observations can improve understanding, they face limitations in spatial resolution, coverage, and frequency. In contrast, fixed in situ measurements calibrated to World Meteorological Organization standards offer high precision continuous data, although with limited spatial coverage due to logistical constraints. This study uses in situ observations from single tower sites in five northeastern United States cities to estimate total urban CH4emissions using a Bayesian scaling factor framework. Despite limited spatial sampling, the approach yields robust emission estimates consistent with other studies. To explore drivers of variability, the analysis examines correlations between inferred emissions and urban characteristics including population, residential gas usage, and infrastructure. Results show that residential building volume outperforms population as a predictor in some regions, highlighting the importance of infrastructure-specific factors. By demonstrating a scalable observation-based approach using minimal sites, this work addresses key gaps in urban CH4monitoring and emphasizes the value of robust measurements and tailored proxies for improving emission estimates in diverse urban settings.
UR - https://www.scopus.com/pages/publications/105010624358
UR - https://www.scopus.com/inward/citedby.url?scp=105010624358&partnerID=8YFLogxK
U2 - 10.1021/acs.est.5c03844
DO - 10.1021/acs.est.5c03844
M3 - Article
C2 - 40633562
AN - SCOPUS:105010624358
SN - 0013-936X
VL - 59
SP - 14399
EP - 14409
JO - Environmental Science and Technology
JF - Environmental Science and Technology
IS - 28
ER -