Templated grain growth of high coercive field CuO-doped textured PYN-PMN-PT ceramics

Michael J. Brova; Beecher H. Watson; Rebecca L. Walton; Elizabeth R. Kupp; Mark A. Fanton; Richard J. Meyer; Gary L. Messing

doi:10.1111/jace.17349

Templated grain growth of high coercive field CuO-doped textured PYN-PMN-PT ceramics

Michael J. Brova, Beecher H. Watson, Rebecca L. Walton, Elizabeth R. Kupp, Mark A. Fanton, Richard J. Meyer, Gary L. Messing

Research output: Contribution to journal › Article › peer-review

15 Scopus citations

Abstract

This paper explores the templated grain growth and texturing of Pb(Yb_1/2Nb_1/2)O₃-Pb(Mg_1/3Nb_2/3)O₃-PbTiO₃ (PYN-PMN-PT) ceramics. A PbO-CuO liquid phase was determined to substantially increase the growth of PYN-PMN-PT on barium titanate template particles. Texturing resulted in an 83% enhancement in strain behavior (754 pm/V) compared with random PYN-PMN-PT ceramics (413 pm/V). The increased Pb(Yb_1/2Nb_1/2)O₃ (PYN) content of textured 21PYN-41PMN-38PT resulted in a high coercive field of 13.9 kV/cm. Residual barium titanate templates reduced the polarization from 33.7 to 26.2 µC/cm² and slightly decreased the Curie temperature (236-224°C). These results show that textured PYN-PMN-PT is a promising material for high strain and coercive field transducers.

Original language	English (US)
Pages (from-to)	6149-6156
Number of pages	8
Journal	Journal of the American Ceramic Society
Volume	103
Issue number	11
DOIs	https://doi.org/10.1111/jace.17349
State	Published - Nov 1 2020

All Science Journal Classification (ASJC) codes

Ceramics and Composites
Materials Chemistry

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@article{070da6fb3aed4bcc858d4b4b60047e59,

title = "Templated grain growth of high coercive field CuO-doped textured PYN-PMN-PT ceramics",

abstract = "This paper explores the templated grain growth and texturing of Pb(Yb1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 (PYN-PMN-PT) ceramics. A PbO-CuO liquid phase was determined to substantially increase the growth of PYN-PMN-PT on barium titanate template particles. Texturing resulted in an 83% enhancement in strain behavior (754 pm/V) compared with random PYN-PMN-PT ceramics (413 pm/V). The increased Pb(Yb1/2Nb1/2)O3 (PYN) content of textured 21PYN-41PMN-38PT resulted in a high coercive field of 13.9 kV/cm. Residual barium titanate templates reduced the polarization from 33.7 to 26.2 µC/cm2 and slightly decreased the Curie temperature (236-224°C). These results show that textured PYN-PMN-PT is a promising material for high strain and coercive field transducers.",

author = "Brova, {Michael J.} and Watson, {Beecher H.} and Walton, {Rebecca L.} and Kupp, {Elizabeth R.} and Fanton, {Mark A.} and Meyer, {Richard J.} and Messing, {Gary L.}",

note = "Publisher Copyright: {\textcopyright} 2020 The American Ceramic Society",

year = "2020",

month = nov,

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doi = "10.1111/jace.17349",

language = "English (US)",

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T1 - Templated grain growth of high coercive field CuO-doped textured PYN-PMN-PT ceramics

AU - Brova, Michael J.

AU - Watson, Beecher H.

AU - Walton, Rebecca L.

AU - Kupp, Elizabeth R.

AU - Fanton, Mark A.

AU - Meyer, Richard J.

AU - Messing, Gary L.

PY - 2020/11/1

Y1 - 2020/11/1

N2 - This paper explores the templated grain growth and texturing of Pb(Yb1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 (PYN-PMN-PT) ceramics. A PbO-CuO liquid phase was determined to substantially increase the growth of PYN-PMN-PT on barium titanate template particles. Texturing resulted in an 83% enhancement in strain behavior (754 pm/V) compared with random PYN-PMN-PT ceramics (413 pm/V). The increased Pb(Yb1/2Nb1/2)O3 (PYN) content of textured 21PYN-41PMN-38PT resulted in a high coercive field of 13.9 kV/cm. Residual barium titanate templates reduced the polarization from 33.7 to 26.2 µC/cm2 and slightly decreased the Curie temperature (236-224°C). These results show that textured PYN-PMN-PT is a promising material for high strain and coercive field transducers.

AB - This paper explores the templated grain growth and texturing of Pb(Yb1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 (PYN-PMN-PT) ceramics. A PbO-CuO liquid phase was determined to substantially increase the growth of PYN-PMN-PT on barium titanate template particles. Texturing resulted in an 83% enhancement in strain behavior (754 pm/V) compared with random PYN-PMN-PT ceramics (413 pm/V). The increased Pb(Yb1/2Nb1/2)O3 (PYN) content of textured 21PYN-41PMN-38PT resulted in a high coercive field of 13.9 kV/cm. Residual barium titanate templates reduced the polarization from 33.7 to 26.2 µC/cm2 and slightly decreased the Curie temperature (236-224°C). These results show that textured PYN-PMN-PT is a promising material for high strain and coercive field transducers.

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Templated grain growth of high coercive field CuO-doped textured PYN-PMN-PT ceramics

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